Comparision of Nitrogen and Phosphorus
Three major features:
- the radius of phosphorus is 50% greater than that
of nitrogen
- the ionization energies decrease from N to P
- the bond energy trends are different
The oxidation states for both elements vary from
+5 to -3,
but the stability trends are different.
Valence shell expansion: the coordination number
of nitorgen
is <= 4, but phosphorus is larger and the C.N.
can be up to 6.
PF6- and PCl6-
but NH4+ and NF4+
Bond enthalpies:
N-H vs P-H chemistry
The N-H bond is stronger than the P-H bond
(386 vs 321 kJmol-l), so despite a lower DHo(atm)
for P,
PH3 is thermodynamically unstable. PH3
is pyrophoric (kinetics). NH3 also a stronger base.
Lone-pair repulsion
Nitrogen:
Weakens N-X bonds in many nitrogen compounds
resulting in thermodynamic instability,
e.g., the oxides and
halides.
Phosphorus:
Much reduced in P-X bonds (also dp-pp
bonding, see below)
hence stronger bonds and thermodynamically
stable halides and oxides.
Compare:
Hydrolysis of NCl3 gives NH3
and Cl2O
whereas PCl3 gives H3PO3
and HCl.
pp-pp
bonding
Nitrogen:
Very important feature of nitrogen chemistry.
Coupled with weak N-X single bonds,
nitrogen compounds tend to be monomeric or dimeric,
e.g., elemental nitrogen (N2), oxides,
nitrates and nitrites.
Phosphorus:
Quite strong multiple bonds but single bonds
even more important.
Hence many phosphorus compounds "polymerize", e.g.,
the oxides (N2O3 and N2O5 vs
P4O6 and P4O10),
oxy-anions, suphides [note: NO is monomeric but N4S4
and P4S3, P4S4 etc],
elemental phosphorus (P4), and nitrogen
compounds [e.g., (NPCl2)4].
dp-pp
bonding
Open only to phosphorus, and particularly in
compounds with the more electronegative elements N, O, F.
Strengthens both P-X and P=X bonds and hence chain
or cyclic structures for the oxides and oxy-anion salts.
Kinetic effects too:
X3N-O X3P=O
Normal N-O bond length; Short P=O bond;
high polarity; low energy; low polarity; high
energy;
high reactivity inert
Oxidation states
- Negative oxidation state stability N > P
- Positive oxidation states P > N
- Oxidation states: NCl3 very unstable
but PCl3 stable;
N2O5, NO3
, NF4 but P4O10, PF5, PCl5,
PBr5; nitric acid
is very oxidizing but phosphoric acid is not.
- In aqueous solution: refer to oxidation state
diagram.
Note: H3PO2 is in fact
H2P(=O)OH, and phosphorous acid is
not P(OH)3 but HP(=O)(OH)2
- an indication of the P=O
bond strength
- Donor properties of NR3 and PR3
in complex formation.